کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
8090924 | 1521984 | 2015 | 10 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Investigation of carbon dioxide capture with aqueous piperazine on a post combustion pilot plant - Part II: Parameter study and emission measurement
دانلود مقاله + سفارش ترجمه
دانلود مقاله ISI انگلیسی
رایگان برای ایرانیان
کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
علوم زمین و سیارات
فرآیندهای سطح زمین
پیش نمایش صفحه اول مقاله
![عکس صفحه اول مقاله: Investigation of carbon dioxide capture with aqueous piperazine on a post combustion pilot plant - Part II: Parameter study and emission measurement Investigation of carbon dioxide capture with aqueous piperazine on a post combustion pilot plant - Part II: Parameter study and emission measurement](/preview/png/8090924.png)
چکیده انگلیسی
This paper continues the investigation of a 37.6Â wt% piperazine solution (7 molal) in a PCC-test facility on the power plant in Dürnrohr, Austria. The use of real power plant flue gas and the well-conceived dimensions of the test facility enable industry-related conditions for full scale applications. A minimum specific energy for solvent regeneration of 3.17Â GJ/tCO2 was determined in Part I of this paper. The optimal solvent flow rate is 20% lower in comparison to that of 30Â wt% MEA. Part II tries to reduce the energy consumption further by carrying out a detailed parameter study. Especially at high flue gas flow rates, piperazine shows a good performance because of its fast kinetics. If the maximum achievable flue gas flow rate of 120Â m3/h (F-factor â¼2Â Pa0.5) is set, the specific energy for solvent regeneration drops to 3Â GJ/tCO2. The fast kinetics has also a positive effect by reduction of the absorber height. Halving the absorber height still allows a performance similar to that of 30Â wt% MEA. Due to the high thermal stability, piperazine enables an operation with high desorber pressures. Higher desorber pressures, resulting in a lower CO2 compression work. In addition, the regeneration energy can be further reduced. An energy saving can also be achieved by the temperature reduction of the incoming flue gas. By operation with flue gases of a natural gas-fired boiler, the minimal energy consumption rises to 3.6Â GJ/tCO2. The optimal solvent flow rate decreases as with 30Â wt% MEA. An emission measurement shows a direct correlation between NH3 concentration of the treated flue gas and the solvent flow rate. Because of low water circulation in the water washing section, the NH3 emissions in the treated flue gas increase at high solvent flow rates.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: International Journal of Greenhouse Gas Control - Volume 37, June 2015, Pages 471-480
Journal: International Journal of Greenhouse Gas Control - Volume 37, June 2015, Pages 471-480
نویسندگان
Markus Rabensteiner, Gerald Kinger, Martin Koller, Günter Gronald, Christoph Hochenauer,