کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
9594609 | 1507971 | 2005 | 15 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Differential probability for surface and volume electronic excitations in Fe, Pd and Pt
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
شیمی
شیمی تئوریک و عملی
پیش نمایش صفحه اول مقاله
![عکس صفحه اول مقاله: Differential probability for surface and volume electronic excitations in Fe, Pd and Pt Differential probability for surface and volume electronic excitations in Fe, Pd and Pt](/preview/png/9594609.png)
چکیده انگلیسی
The normalized differential mean free path for volume scattering and the differential surface excitation probability for medium energy electrons travelling in Fe, Pd and Pt are extracted from reflection electron energy loss spectra (REELS). This was achieved by means of a recently introduced procedure in which two REELS spectra taken under different experimental conditions are simultaneously deconvoluted. In this way, it is possible to obtain the unique reconstruction for the surface and volume single scattering loss distribution. The employed method is compared with a procedure that is frequently used for this purpose [S. Tougaard, I. Chorkendorff, Phys. Rev. B 35 (1987) 6570]. It is shown, both theoretically and through analysis of model spectra as well as experimental data that the approach by Tougaard and Chorkendorff does not result in a single scattering loss distribution. Rather, it gives a mixture of surface, bulk and mixed scattering of any order.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Surface Science - Volume 588, Issues 1â3, 20 August 2005, Pages 26-40
Journal: Surface Science - Volume 588, Issues 1â3, 20 August 2005, Pages 26-40
نویسندگان
Wolfgang S.M. Werner,