کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
1564653 | 1514170 | 2016 | 7 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Investigation of the sintering of barytocalcite with BaCO3 as a secondary phase for immobilizing carbon-14
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
مهندسی انرژی
انرژی هسته ای و مهندسی
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چکیده انگلیسی
The effect of a secondary phase (BaCO3) on the sintering of synthetic barytocalcite has been investigated. It was found that this phase impacts the sintering positively by lowering the sintering activation energy from 230 to 160Â kJÂ molâ1, by increasing the shrinkage rate and by reaching higher densities. However, BaCO3, originally dispersed in the powder, was segregated by diffusion during sintering with a large part of it being located at the grain boundaries. The dense pellet is made of both phases barytocalcite and BaCO3, what should be avoided to give the best leaching resistance. Thus the BaCO3 presence should be limited as much as possible by controlling the reactants stoichiometry during the synthesis.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Journal of Nuclear Materials - Volume 476, 1 August 2016, Pages 13-19
Journal: Journal of Nuclear Materials - Volume 476, 1 August 2016, Pages 13-19
نویسندگان
Nicolas Massoni, Sophie Le Gallet,