کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
1568580 | 999900 | 2008 | 6 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Dissolution of uranium metal without hydride formation or hydrogen gas generation
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
مهندسی انرژی
انرژی هسته ای و مهندسی
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چکیده انگلیسی
This study shows that metallic uranium will cleanly dissolve in carbonate-peroxide solution without generation of hydrogen gas or uranium hydride. Metallic uranium shot, 0.5–1 mm diameter, was reacted with ammonium carbonate–hydrogen peroxide solutions ranging in concentration from 0.13 M to 1.0 M carbonate and 0.50 M to 2.0 M peroxide. The dissolution rate was calculated from the reduction in bead mass, and independently by uranium analysis of the solution. The calculated dissolution rate ranged from about 4 × 10−3 to 8 × 10−3 mm/h, dependent primarily on the peroxide concentration. Hydrogen analysis of the etched beads showed that no detectable hydrogen was introduced into the uranium metal by the etching process.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Journal of Nuclear Materials - Volume 378, Issue 3, 1 September 2008, Pages 299–304
Journal: Journal of Nuclear Materials - Volume 378, Issue 3, 1 September 2008, Pages 299–304
نویسندگان
Chuck Soderquist, Bruce McNamara, Brian Oliver,