کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
4364649 | 1616318 | 2015 | 8 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Degradation of a broad spectrum of trace organic contaminants by an enzymatic membrane reactor: Complementary role of membrane retention and enzymatic degradation
ترجمه فارسی عنوان
تخریب طیف گسترده ای از آلاینده های آلاینده های آلاینده توسط یک راکتور غشایی آنزیمی: نقش مکمل نگهداری غشاء و تخریب آنزیمی
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کلمات کلیدی
موضوعات مرتبط
علوم زیستی و بیوفناوری
علوم محیط زیست
علوم زیست محیطی (عمومی)
چکیده انگلیسی
Laccase-catalysed degradation of 30 trace organic contaminants (TrOCs) with diverse chemical structure was investigated in an enzymatic membrane reactor (EMR) equipped with an ultrafiltration membrane. Compared to the results from batch incubation tests, the EMR could facilitate degradation of some phenolic and a number of non-phenolic TrOCs. Laccase, which was completely retained by the membrane, formed a dynamic gel layer on the membrane surface onto which TrOCs were adsorbed. EMR investigations with active and heat-inactivated laccase confirmed that the TrOCs retained by the active laccase gel layer were eventually degraded. Redox-mediator addition to the EMR significantly extended the spectrum of efficiently degraded TrOCs, but a limited improvement was observed in batch tests. The results demonstrate the important role of TrOC retention by the enzyme gel layer dynamically formed on the membrane in achieving improved degradation of TrOCs by the mediator-assisted laccase system. Despite following the same hydrogen atom transfer pathway, the mediators tested (syringaldehyde and 1-hydroxybenzotriazole) exhibited TrOC-specific degradation improvement capacity.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: International Biodeterioration & Biodegradation - Volume 99, April 2015, Pages 115-122
Journal: International Biodeterioration & Biodegradation - Volume 99, April 2015, Pages 115-122
نویسندگان
Luong N. Nguyen, Faisal I. Hai, William E. Price, Jinguo Kang, Frederic D.L. Leusch, Felicity Roddick, Jason P. van de Merwe, Saleh F. Magram, Long D. Nghiem,