The effect of rain characteristics on scavenging rate of tritium-oxide from the atmosphere

The results of field experiments, involving HTO scavenging from the atmosphere by precipitation in the vicinity of HT and HTO emission sources, are presented. The experiments were aimed at obtaining direct experimental data on atmospheric HTO scavenging for a variety of rain characteristics (rain intensity and drop spectra).The most reliable are the calculations of the rate of wash-out with precipitation with the use of the method of integration of the constant exchange for a spectrum of drops. The results of such calculations are in good agreement with the experimental data and can serve as a basis for the generalized parameterization dependences. It is shown that the exact calculation can be replaced by a simpler formula using the mean-value theorem.For the known approximations of the spectra of the rain drops, formulas were obtained to give parameterization dependence of the rate of wash-out Λ on the intensity of precipitation p. This approach can be used for rapid assessment, as well as to determine parameters of wash-out of gases with precipitation in the numerical complexes, which are used for the calculation of the transfer and removal of impurities from the atmosphere.

► The results of field experiments in HTO scavenging with precipitations from the atmosphere are presented.
► The precipitation parameters were experimentally measured, the drop spectra were processed.
► The comparison of the calculations with the results has shown a good agreement.
► The model was developed to calculate scavenging rates for arbitrary drop spectra.
► The parameterized dependence for the Λ scavenging rate on precipitation intensity p was proposed.