کد مقاله کد نشریه سال انتشار مقاله انگلیسی نسخه تمام متن
4994126 1458030 2017 16 صفحه PDF دانلود رایگان
عنوان انگلیسی مقاله ISI
Design and optimization of substrate placement for large-sized and high-quality fused silica glass by SiCl4 flame hydrolysis deposition
موضوعات مرتبط
مهندسی و علوم پایه مهندسی شیمی جریان سیال و فرایندهای انتقال
پیش نمایش صفحه اول مقاله
Design and optimization of substrate placement for large-sized and high-quality fused silica glass by SiCl4 flame hydrolysis deposition
چکیده انگلیسی
This paper presents numerical studies of large-size and high-quality fused silica glass synthesis by SiCl4 flame hydrolysis deposition method, specifically the correlation of uniformities of SiO2 deposition and OH concentration with the optimal location of the substrate placement. A comprehensive computational model is developed to describe the complex turbulent reacting flow with the detailed SiCl4-H2-O2 reaction mechanism. Numerical simulation is first conducted to obtain the characteristics of SiCl4 hydrolysis flame without considering the substrate and the SiO2 particle formation. The distribution of SiO2 accumulation is then calculated. The potential region and location for placing substrate are initially determined based on the criterion of a uniform SiO2 accumulation. Further, the effects of H2-O2 equivalence ratio and the SiCl4 flow rate on the distributions of the temperature, SiO2 concentration and OH concentration are investigated. It is found that the H2-O2 equivalence ratio is sensitive to the temperature and the OH concentration, and the flow rate of SiCl4 mainly affects the temperature and SiO2 concentration. This finding indicates that the H2-O2 equivalence ratio and the flow rate of SiCl4 have equally important roles in determining the optimal location for the deposition substrate placement. The presence of the substrate also changes the distributions of the temperature and compositions concentrations in the furnace. Adjusting the substrate location is an effective strategy to achieve optimal location with more uniform distributions of the SiO2 accumulation and the OH concentration on the deposition surface.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: International Journal of Heat and Mass Transfer - Volume 111, August 2017, Pages 917-932
نویسندگان
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