کد مقاله کد نشریه سال انتشار مقاله انگلیسی نسخه تمام متن
5432236 1508831 2017 11 صفحه PDF دانلود رایگان
عنوان انگلیسی مقاله ISI
In-situ neutron imaging of hydrogenous fuels in combustion generated porous carbons under dynamic and steady state pressure conditions
ترجمه فارسی عنوان
تصویربرداری نوترونی در سوختهای هیدروژنی در احتراق موجب تولید کربن متخلخل تحت شرایط فشار پویا و حالت پایدار
موضوعات مرتبط
مهندسی و علوم پایه مهندسی انرژی انرژی (عمومی)
چکیده انگلیسی

We report results from experiments where we characterize the surface properties of soot particles interacting with high-pressure methane. We find considerable differences in behavior of the soot material between static and dynamic pressure conditions that can be explained by multiscale correlations in the dynamics, from the micro to macro of the porous fractal-like carbon matrix. The measurements were possible utilizing cold neutron imaging of methane mixed with combustion generated carbon (soot) inside steel cells. The studies were performed under static and dynamic pressure conditions in the range 10–90 bar, and are of interest for applications of energy storage of hydrogenous fuels. The very high cross sections for neutrons compared to hard X-ray photons, enabled us to find considerable amounts of native hydrogen in the soot and to see and quantify the presence of hydrogen atoms in the carbon soot matrix under different pressure conditions. This work lays the base for more detailed in-situ investigations on the interaction of porous carbon materials with hydrogen in practical environments for hydrogen and methane storage.

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ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Carbon - Volume 116, May 2017, Pages 766–776