کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
7721026 | 1497511 | 2013 | 10 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Effect of CaO on tar reforming to hydrogen-enriched gas with in-process CO2 capture in a bubbling fluidized bed biomass steam gasifier
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
شیمی
الکتروشیمی
پیش نمایش صفحه اول مقاله
![عکس صفحه اول مقاله: Effect of CaO on tar reforming to hydrogen-enriched gas with in-process CO2 capture in a bubbling fluidized bed biomass steam gasifier Effect of CaO on tar reforming to hydrogen-enriched gas with in-process CO2 capture in a bubbling fluidized bed biomass steam gasifier](/preview/png/7721026.png)
چکیده انگلیسی
Previous studies showed that calcium oxide (CaO), when added to a biomass steam gasifier, could play the role of both CO2 sorbent and tar reforming catalyst, and thereby produce more hydrogen. However, most of these works focused on the former role with little attention to tar reforming aspect of CaO. Therefore, this work aims primarily at studying the tar reforming effect of in-bed CaO. To this end, an in-depth analysis of the effect of CaO on tar yield and composition is presented. The present work also studies the role of CaO as a CO2 sorbent to enhance hydrogen production from steam gasification of biomass in a bubbling fluidized bed. The influence of different operating parameters, temperature (T) and steam to biomass (S/B) ratio, as well as the effect of using in-bed CaO on gas and tar production is investigated. Results show that the maximum H2 and minimum CO2 concentration of 63.07% and 18.68%, respectively are obtained at T = 650 °C and S/B = 3.41. The maximum H2 yield of 256.81 ml gâ1-biomass was obtained at T = 700 °C and S/B = 3.41, at which the minimum tar content of 6.45 g N mâ3 was also received. Compared to a bed of sand alone, a 20% higher H2 concentration, an almost double H2 yield and a 67% reduction in tar content were obtained when a bed of CaO was used. Moreover, shifting the tar species from higher to fewer ring structures as a result of in-bed CaO can reduce tar dew point by 11 °C and tar carcinogenic potential by almost 60%.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: International Journal of Hydrogen Energy - Volume 38, Issue 34, 13 November 2013, Pages 14495-14504
Journal: International Journal of Hydrogen Energy - Volume 38, Issue 34, 13 November 2013, Pages 14495-14504
نویسندگان
Jakkapong Udomsirichakorn, Prabir Basu, P. Abdul Salam, Bishnu Acharya,