کد مقاله کد نشریه سال انتشار مقاله انگلیسی نسخه تمام متن
8863814 1620291 2018 9 صفحه PDF دانلود رایگان
عنوان انگلیسی مقاله ISI
Global gridded anthropogenic emissions inventory of carbonyl sulfide
ترجمه فارسی عنوان
موجودی انبساط کربونیل سولفید جهانی را در بر می گیرد
کلمات کلیدی
کربنیل سولفید، انسان شناسی، جهانی، منابع اتمسفر،
موضوعات مرتبط
مهندسی و علوم پایه علوم زمین و سیارات علم هواشناسی
چکیده انگلیسی
Atmospheric carbonyl sulfide (COS or OCS) is the most abundant sulfur containing gas in the troposphere and is an atmospheric tracer for the carbon cycle. Gridded inventories of global anthropogenic COS are used for interpreting global COS measurements. However, previous gridded anthropogenic data are a climatological estimate based on input data that is over three decades old and are not representative of current conditions. Here we develop a new gridded data set of global anthropogenic COS sources that includes more source sectors than previously available and uses the most current emissions factors and industry activity data as input. Additionally, the inventory is provided as annually varying estimates from years 1980-2012 and employs a source specific spatial scaling procedure. We estimate a global source in year 2012 of 406 Gg S y−1 (range of 223-586 Gg S y−1), which is highly concentrated in China and is twice as large as the previous gridded inventory. Our large upward revision in the bottom-up estimate of the source is consistent with a recent top-down estimate based on air-monitoring and Antarctic firn data. Furthermore, our inventory time trends, including a decline in the 1990's and growth after the year 2000, are qualitatively consistent with trends in atmospheric data. Finally, similarities between the spatial distribution in this inventory and remote sensing data suggest that the anthropogenic source could potentially play a role in explaining a missing source in the global COS budget.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Atmospheric Environment - Volume 183, June 2018, Pages 11-19
نویسندگان
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