کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
9595075 | 1507966 | 2005 | 6 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Two-photon photoemission from silver nanoparticles on thin alumina films: Role of plasmon excitation
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
شیمی
شیمی تئوریک و عملی
پیش نمایش صفحه اول مقاله
چکیده انگلیسی
Two-photon photoemission (2PPE) from silver nanoparticles on a thin Al2O3 film on NiAl(1Â 1Â 0) has been investigated using femtosecond lasers. The 2PPE spectra show a feature similar to the surface state of Ag(1Â 1Â 1). The total 2PPE yield possesses a maximum at about 3.6Â eV which corresponds to the surface plasmon resonance of the silver particles. For particle sizes of about 10Â nm an enhancement by a factor 450 compared to Ag(1Â 1Â 1) is found. Up to this diameter the photoemission yield increases but levels off for larger sizes due to interactions between the particles. It is inferred that the 2PPE process is a direct transition via a virtual state, and that the enhanced 2PPE yield results from the enhancement of the electromagnetic field at the surface of nanoparticles.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Surface Science - Volume 593, Issues 1â3, 20 November 2005, Pages 43-48
Journal: Surface Science - Volume 593, Issues 1â3, 20 November 2005, Pages 43-48
نویسندگان
Florian Evers, Christoph Rakete, Kazuo Watanabe, Dietrich Menzel, Hans-Joachim Freund,