کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
11000309 | 1423540 | 2018 | 9 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Experimental and numerical study of OH* chemiluminescence in hydrogen diffusion flames
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
مهندسی شیمی
مهندسی شیمی (عمومی)
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چکیده انگلیسی
A co-flow burner was designed to generate axisymmetric diffusion flames for the application of line-of-sight optical diagnostics to hydrogen flames. Chemiluminescence images of OH* from laminar hydrogen diffusion flames, with and without co-flowing air, were recorded using an intensified camera system with a narrow-band filter at approximately 310 nm. The spectra of OH* chemiluminescence was acquired by a separate optical system. Local concentrations of the radiating radical OH* were determined using the inverse Abel transformation and calibration against a light source of known radiance. The uncertainty of the OH* concentration measurements is analysed to be â22% to +12% in the current experimental configuration. Numerical reconstruction of the physical flames was performed using a two dimensional axisymmetric flow model coupled with a detailed H2/O2 oxidation chemistry mechanism and an OH* chemiluminescent sub-scheme which includes options to use 6 different rate coefficients recommended in the literature for the OH* formation reaction H+O+MâOH*+M (R1). The numerical simulations using the rate coefficient of 1.5â¯Ãâ¯1013exp(â5.98kcalmolâ1/RT)cm6molâ2sâ1 for R1 demonstrate the best agreement with the measured OH* chemiluminescence.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Combustion and Flame - Volume 197, November 2018, Pages 369-377
Journal: Combustion and Flame - Volume 197, November 2018, Pages 369-377
نویسندگان
Mengmeng Zhao, David Buttsworth, Rishabh Choudhury,