کد مقاله کد نشریه سال انتشار مقاله انگلیسی نسخه تمام متن
1239831 1495721 2012 8 صفحه PDF دانلود رایگان
عنوان انگلیسی مقاله ISI
Numerical and experimental investigation of laser induced plasma spectrum of aluminum in the presence of a noble gas
موضوعات مرتبط
مهندسی و علوم پایه شیمی شیمی آنالیزی یا شیمی تجزیه
پیش نمایش صفحه اول مقاله
Numerical and experimental investigation of laser induced plasma spectrum of aluminum in the presence of a noble gas
چکیده انگلیسی

Laser-induced plasma emission of an aluminum target in helium gas at 1 atm pressure is numerically and experimentally investigated. A laser pulse at wavelength of 266 nm and pulse duration of 10 ns has been considered. Laser ablation is calculated by a one dimensional model based on thermal evaporation mechanism. Spatial and temporal parameters of plasma expansion are determined by using hydrodynamic equations. Three kinds of plasma emission, including Bremsstrahlung, recombination and spectral emissions are considered for modeling the spectrum. Strong lines of aluminum and helium in wavelength interval of 200 to 450 nm are selected. Aluminum spectrum in UV range is depicted and compared with other spectral ranges. Temporal and spatial evolution of plasma emission up to 200 ns after the laser irradiation is studied. The effect of laser energy on the plasma spectrum is studied. An experimental set-up is arranged to compare numerical calculations with experimental results. Experimental and numerical results illustrate that helium line widths and peak intensities become narrower and weaker with time, respectively. Spatial distribution of spectrum shows that for closer distance to the sample surface, an intense continuous emission is observed, while at the farther distance, continuous emission decreases and spectral lines become sharper. A good coincidence is observed between experimental and numerical results.


► Aluminum plasma emission in helium is numerically and experimentally studied.
► Spectral, Bremsstrahlung and recombination emissions in spectrum are calculated.
► All strong lines of aluminum and helium are chosen for spectrum simulation.
► Line widths and peak intensities at later times become narrower and weaker.
► At specific optimum position, the maximum of signal peaks is acquired.

ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Spectrochimica Acta Part B: Atomic Spectroscopy - Volume 78, 1 December 2012, Pages 29–36
نویسندگان
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