کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
1283464 | 1497640 | 2009 | 6 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Dark and acidic conditions for fermentative hydrogen production
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
شیمی
الکتروشیمی
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چکیده انگلیسی
Bacterial consortium capable of producing hydrogen in low pH (LpH) range of 3.3-4.3 is reported in this study. This operational pH is two full units below that of previously reported hydrogen producing organisms. Low pH inocula were derived from a batch biohydrogen reactor inoculated with heat treated compost (â¼120 °C, 2 h), which was allowed to accumulate biogas to reach three atmospheres of equivalent headspace pressure and system pH of 3.0. Acclimation effect had positive influence on H2 production and LpH inocula were passed sequentially into more than 15 generations to achieve consistent conversion efficiency and hydrogen composition, further tested in 23 other culture cycles. With hydrogen composition in the headspace ranging from 50% to 60%, conversion efficiency of â¼43% achieved in LpH systems is comparable to that of other buffered systems. Feasibility of hydrogen production in LpH systems is demonstrated in unbuffered reactors under intermittent pressure release conditions and in absence of initial pH adjustment and stirring. Conversion efficiencies, however, decreased by â¼1-fold for each 3 °C drop below the optimum temperature of 22 °C.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: International Journal of Hydrogen Energy - Volume 34, Issue 2, January 2009, Pages 821-826
Journal: International Journal of Hydrogen Energy - Volume 34, Issue 2, January 2009, Pages 821-826
نویسندگان
Venkataramana Gadhamshetty, David C. Johnson, Nagamany Nirmalakhandan, Geoff B. Smith, Shuguang Deng,