کد مقاله کد نشریه سال انتشار مقاله انگلیسی نسخه تمام متن
5396933 1505772 2007 5 صفحه PDF دانلود رایگان
عنوان انگلیسی مقاله ISI
One-photon two-electron processes in helium: Unity and diversity
موضوعات مرتبط
مهندسی و علوم پایه شیمی شیمی تئوریک و عملی
پیش نمایش صفحه اول مقاله
One-photon two-electron processes in helium: Unity and diversity
چکیده انگلیسی
The ab initio HRM-SOW method has established itself as the ideally fit tool to explore the three-body dynamics of the helium atom close to its full break-up threshold. Accordingly, it is used here to perform a “numerical experiment” designed to enlighten the relations between the various competing processes which may occur in the vicinity of the double ionization threshold, be it double excitation, excitation-ionization, or double ionization. More precisely, double ionization and ionization-excitation cross-sections are produced at 100 meV above the double ionization threshold. The latter, obtained up to as high a level as n=50, are in addition analyzed in terms of spherical and parabolic partial waves in the photo-electron frame. Based on these extensive data, we establish a continuity relation between ionization-excitation and double ionization appropriate to the near threshold region, confirm previous qualitative predictions regarding the dominant angular momentum achieved in these near threshold excitation processes, evidence the relation between ionized-excited and doubly excited states, and promote the partial parabolic ionization-excitation cross-sections as the optimal observation channels of doubly excited states.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Journal of Electron Spectroscopy and Related Phenomena - Volume 161, Issues 1–3, October 2007, Pages 80-84
نویسندگان
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