کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
5399302 | 1505892 | 2015 | 7 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Influence of defects on sub-Ã
optical linewidths in Eu3+: Y2O3 particles
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
شیمی
شیمی تئوریک و عملی
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چکیده انگلیسی
Rare earth doped nanocrystals have been recently suggested as useful materials for applications in quantum information processing. To reach optical properties closer to bulk crystals ones, it is still necessary to reduce the defects that can arise in nanoscale structures. Here, we probe the defects level by monitoring the inhomogeneous broadening of the 7F0â5D0 transition in particles of 0.3% at% Eu3+:Y2O3. We find that lines as narrow as 14 GHz (0.015 nm), a value comparable to single crystals, can be obtained in 150 nm particles calcinated at 1200 °C. The additional broadening observed for particles calcinated at lower temperature is attributed to defects inside crystallites and not to surface effects. A linear correlation is also observed between optical and Raman linewidths, suggesting that both processes are sensitive to the same defects. 5D0 excited state lifetimes are well described by a model based on an effective refractive index and we conclude that the defects causing the inhomogeneous broadening have no effect on the excited state population.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Journal of Luminescence - Volume 168, December 2015, Pages 276-282
Journal: Journal of Luminescence - Volume 168, December 2015, Pages 276-282
نویسندگان
Karmel de Oliveira Lima, Rogéria Rocha Gonçalves, Domitille Giaume, Alban Ferrier, Philippe Goldner,