Generation of widely tunable Fourier-transform-limited terahertz pulses using narrowband near-infrared laser radiation

Widely tunable, Fourier-transform-limited pulses of terahertz (THz) radiation have been generated using (i) crystals of the highly nonlinear organic salt 4-N,N-dimethylamino-4′-N′-methyl stilbazolium tosylate (DAST), (ii) zinc telluride (ZnTe) crystals, (iii) gallium phosphide (GaP) crystals, and (iv) low-temperature-grown gallium arsenide (LTG-GaAs) photomixers with THz spiral antennas. Outputs from two narrowband (Δν < 1 MHz, λ ∼ 800 nm) cw titanium-doped sapphire (Ti:Sa) ring lasers with a well-controlled frequency difference were shaped into pulses using acousto-optic modulators (AOM), coupled into an optical fiber, pulse amplified in Nd:YAG-pumped Ti:Sa crystals and used as optical sources to pump the THz emitters. The THz radiation was detected over a broad frequency range and its bandwidth was determined to be ∼10 MHz. The spectroscopic potential of the THz source is illustrated by the absorption spectrum of a pure rotational transition of OCS.