کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
6611873 | 459565 | 2015 | 9 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Enhancing the Efficiency and Charge Transport Characteristics of Dye-Sensitized Solar Cells by Adding Graphene Nanosheets to TiO2 Working Electrodes
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
مهندسی شیمی
مهندسی شیمی (عمومی)
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چکیده انگلیسی
In this study, TiO2-GN nanocomposite working electrodes were fabricated by adding graphene nanosheets (GNs) to TiO2 thin-film working electrodes. The influence of the thickness of the TiO2 thin-film working electrodes on the efficiency and charge transport characteristics of the corresponding dye-sensitized solar cells (DSSCs) was investigated. A GN solution was spin-coated onto the TiO2 thin films, which were then sintered at 100 °C in order to fabricate TiO2-GN working electrodes. The characteristics of various working electrodes were analyzed via scanning electron microscopy, atomic force microscopy, surface profilometry, energy-dispersive X-ray spectroscopy, X-ray photoelectron spectroscopy, X-ray diffraction, and Raman spectroscopy. Moreover, the DSSCs fabricated from these working electrodes were characterized via current density-voltage, incident photo-to-current conversion efficiency, electrochemical impedance spectroscopy, intensity-modulated photocurrent spectroscopy, and intensity-modulated photovoltage spectroscopy measurements. The results indicate that adding GNs to TiO2 thin films can enhance the electron transport rate and charge collection efficiency in TiO2-GN working electrodes, and thereby increase the power conversion efficiency of DSSCs. As such, DSSCs containing the TiO2-GN working electrodes exhibited an efficiency of 8.07%, which is 24.3% higher than that (6.49%) of the DSSCs containing conventional TiO2 working electrodes.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Electrochimica Acta - Volume 165, 20 May 2015, Pages 356-364
Journal: Electrochimica Acta - Volume 165, 20 May 2015, Pages 356-364
نویسندگان
Chih-Hung Tsai, Po-Hsi Fei, Wei-Chien Wu,