کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
6974055 | 1453322 | 2018 | 11 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Characterization of new potassium-based solid sorbents prepared using metal silicates for post-combustion CO2 capture
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
مهندسی شیمی
بهداشت و امنیت شیمی
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چکیده انگلیسی
Potassium-based sorbents prepared using metal oxides as supports or additive materials are commonly applied in fast fluidized bed reactors for post-combustion CO2 capture. However, they have some disadvantages in terms of regeneration properties. To overcome these drawbacks, novel potassium-based sorbents, herein termed KAS, KCS, and KZS, prepared using aluminum silicate, calcium silicate, and zirconium silicate, respectively, were developed in this study. Unlike potassium-based sorbents prepared using metal oxides, the new sorbents exhibited high CO2 capture capacities (90-96 mg CO2/g sorbent) and excellent regeneration ratios of 90% or more during multiple tests, even at a the low regeneration temperature of 200 °C. These improved results were achieved because KHCO3 alone is formed during CO2 sorption without any by-product formation, and there is no loss of the active material (K2CO3) during preparation. Thus, metal silicates can be used to prepare potassium-based solid sorbents for CO2 capture at low temperatures.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Process Safety and Environmental Protection - Volume 117, July 2018, Pages 296-306
Journal: Process Safety and Environmental Protection - Volume 117, July 2018, Pages 296-306
نویسندگان
Min Sun Cho, Soo Chool Lee, Ho Jin Chae, Yong Mok Kwon, Joong Beom Lee, Jae Chang Kim,