Measurement of laminar burning velocity and Markstein length relative to fresh gases using a new postprocessing procedure: Application to laminar spherical flames for methane, ethanol and isooctane/air mixtures

The purpose of this study is to present a new tool for extracting the laminar burning velocity in the case of spherically outward expanding flames. This new procedure makes it possible to determine the laminar burning velocity directly based on the flame displacement speed and the global fresh gas velocity near the preheat zone of the flame front. It therefore presents a very interesting alternative to the standard method (commonly used in the literature), which is based on the flame front displacement and the ratio of unburned and burned gas densities. The influence of external flame stretching on the burning velocity can be characterized and the Markstein length relative to the unburned gases (i.e., fresh gases) can be deduced by using this new tool. Contrary to the standard procedure, the unstretched laminar burning velocity is determined directly without using the fuel mixture properties. The temporal evolution of the flame front is visualized by high-speed laser tomography and the algorithm, based on a tomographic image correlation method, makes it possible to accurately measure the fresh gas velocity near the preheat zone of the flame front. The measurements of laminar flame speeds are carried out in a high-pressure and high-temperature constant-volume vessel over a wide range of equivalence ratios for methane, ethanol, and isooctane/air mixtures. To validate the experimental facility and the postprocessing of the flame images, fresh gas velocities and unstretched laminar burning velocities, as well as Markstein lengths relative to burned and unburned gases, are presented and compared with experimental and numerical results of the literature for methane/air flames. New results concerning ethanol/air and isooctane/air flames are presented for various experimental conditions (373 K, equivalence ratios range 0.7–1.5, pressure range 0.1–5 MPa).