A general formulation of monotonically convergent algorithms in the control of quantum dynamics beyond the linear dipole interaction

This paper presents a general method to formulate monotonically convergent algorithms for identifying optimal control fields to manipulate quantum dynamics phenomena beyond the linear dipole interaction. The method, facilitated by a field-dependent dipole moment operator, is based on an integral equation of the first kind arising from the Heisenberg equation of motion for tracking a time-dependent, dynamical invariant observable associated with a reference control field.