کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
5117090 | 1378115 | 2016 | 6 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
The electro/Fe3+/peroxydisulfate (PDS) process coupled to activated sludge culture for the degradation of tetracycline
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
مهندسی انرژی
انرژی های تجدید پذیر، توسعه پایدار و محیط زیست
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چکیده انگلیسی
The removal of tetracycline (TC) by electro/Fe3+/peroxydisulfate process combined to the biological treatment is reported in this study. Effect of current density, peroxydisulfate (PDS) concentration, Fe3+ ions concentration and initial tetracycline concentration were investigated. The results indicated that the removal efficiency of TC increased with increasing current density and decreases with tetracycline initial concentration. This effect is attributed to the competition of TC and electrogenerated intermediate compounds for the consumption of oxidizing SO4â radicals. The TC degradation efficiency was improved significantly when the PDS and Fe3+ concentrations increased from 1 to 10Â mM and 1-2Â mM, respectively. Above 10Â mM PDS and 2Â mM Fe3+ concentrations, a decrease of TC degradation efficiency was observed. The optimal operating conditions were: 2Â mM Fe3+, 0.06Â mMÂ TC, 10Â mM PDS concentrations and 40Â mAÂ cmâ2 current density. Under these conditions a total degradation of TC within only 40Â min of reaction time and 98% of mineralization yield after 3Â h electrolysis were obtained. The biodegradability of the solution after electro/Fe3+/peroxydisulfate pre-treatment showed that BOD5/COD ratio increased from 0.00 initially to 0.42, 0.46 and 0.83 after 4Â h, 5Â h and 6Â h, respectively, namely above the limit of biodegradability (0.4). The enhancement of biodegradability initially from 0.00 to 0.42 and 0.46 after 4Â h and 5Â h of electrolysis respectively, was confirmed by the biological treatment, since 77.51% and 92.54% of the dissolved organic carbon was removed respectively by coupling Electro/Fe3Â +/PDS pre-treatment and a biological treatment.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Journal of Environmental Management - Volume 184, Part 2, 15 December 2016, Pages 249-254
Journal: Journal of Environmental Management - Volume 184, Part 2, 15 December 2016, Pages 249-254
نویسندگان
Amina Ledjeri, Idris Yahiaoui, Farida Aissani-Benissad,