کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
7058133 | 1458076 | 2013 | 7 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Breakdown of Wiedemann-Franz law in individual suspended polycrystalline gold nanofilms down to 3Â K
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
مهندسی شیمی
جریان سیال و فرایندهای انتقال
پیش نمایش صفحه اول مقاله
چکیده انگلیسی
Metallic nanofilms are of great importance in integrated circuit design and electronic devices. Understanding energy dissipation and transport in metallic nanofilms is essential to practical thermal management. The Wiedemann-Franz (WF) law states a precisely fixed ratio by which the electrons transport heat and charge, providing a basic rule to determine the thermal properties. Hitherto no bulk material has been known to violate the WF law. We report compelling evidence for the breakdown of the WF law in polycrystalline gold nanofilms at low temperatures, the Lorenz number increases notably with decreasing temperature. Our results show that the electrons dominate in heat transport at high temperatures, leading to a constant Lorenz number. While below 40Â K, inelastic electron scattering at grain boundaries becomes significant and part of the electron energy is transferred to phonons. Correspondingly, the phonon thermal conductivity is increased and the WF law is violated. A detailed kinetic theoretical model has been developed to investigate several phonon scattering mechanisms in depth and matches well with the experimental results.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: International Journal of Heat and Mass Transfer - Volume 66, November 2013, Pages 585-591
Journal: International Journal of Heat and Mass Transfer - Volume 66, November 2013, Pages 585-591
نویسندگان
Haidong Wang, Jinhui Liu, Xing Zhang, Koji Takahashi,