کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
5404211 | 1505932 | 2006 | 8 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
Laser excitation and excited state dynamics in vanadium dioxide thin film
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
شیمی
شیمی تئوریک و عملی
پیش نمایش صفحه اول مقاله
چکیده انگلیسی
Laser-induced ultrafast nonlinear optical (NLO) response was observed in transient absorption, reflection and NLO measurements in VO2 thin films. The films were prepared using pulsed laser deposition technique with metallic vanadium and V2O5 powder employed as target material. The obtained thin films exhibit a thermal, as well as a laser-induced phase transition (PT) from semiconductor state at room temperature to metallic state. A typical hysterisis was observed for electric resistivity and optical reflectance verses temperature T. For the laser-induced PT in femtosecond pump-probe experiment, the PT was found to be ultrafast, immediately upon laser excitation. Kinetics study suggests that the PT is realized via an intermediate state, presumably a Wannier-Mott exciton (WME) state, followed by a resonant transition to the metallic phase state. The presence of the intermediate state is responsible for an extremely large third-order susceptibility observed in a nonlinear holographic experiment. In a 80Â nm thick VO2 thin amorphous film, the value of Ï(3) was measured to be 1.3Ã10â8Â esu which is four orders of magnitude greater than a standard reference sample of CS2. In addition, the nonlinear response was further enhanced with diffraction signal increased by a factor of 4 after the laser excitation. A signal dip at â¼1.2Â ns was repeatedly observed, which is presumably due to the excitation process associated with the intermediate state. Finally, the resonant transition from the intermediate state to the metallic state, giving rise to a maximum diffraction signal intensity from the formed transient grating.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Journal of Luminescence - Volumes 119â120, JulyâOctober 2006, Pages 404-411
Journal: Journal of Luminescence - Volumes 119â120, JulyâOctober 2006, Pages 404-411
نویسندگان
H. Liu, S. Lysenko, A. Rua, V. Vikhnin, G. Zhang, O. Vasquez, F.E. Fernandez,