کد مقاله | کد نشریه | سال انتشار | مقاله انگلیسی | نسخه تمام متن |
---|---|---|---|---|
9791142 | 1513259 | 2005 | 8 صفحه PDF | دانلود رایگان |
عنوان انگلیسی مقاله ISI
EPR study on magnetic Zn1âxMnxO
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کلمات کلیدی
موضوعات مرتبط
مهندسی و علوم پایه
مهندسی مواد
مواد الکترونیکی، نوری و مغناطیسی
پیش نمایش صفحه اول مقاله
چکیده انگلیسی
Diluted magnetic semiconductors (DMS), systems formed by replacing cations of the host semiconductor material with transition-metal ions, are developed for further use in spintronics. A good combination as a DMS is Zn1âxMnxO due to the ZnO wide band gap (3.37Â eV) and the matching ionic radii of Mn2+ and Zn2+. Using electron paramagnetic resonance we determined the valence of Mn ions in Zn1âxMnxO thin films to be 2+. This is required for explaining the origin of the room temperature ferromagnetism observed in Zn1âxMnxO films. We studied films grown on c-plane sapphire substrates by pulsed laser deposition with the Mn content ranging from x=0.001 to x=0.091 and a single crystal with x=0.035 for comparison. We observed the hyperfine and fine-structure lines of Mn2+ for x=0.001, while for higher Mn contents the fine-structure lines were broadened by dipolar interactions and onto these lines a very broad single line, due to Mn ions in higher local concentrations, was superposed. We modeled the experimental spectra and separated the broad single line from the hyperfine and fine-structure lines. The hyperfine and fine-structure parameters obtained have values characteristic for Zn1âxMnxO lattice sites. We found that the D fine-structure parameter depends on the lattice distortion and Mn content. For example |D| amounts to 675Â MHz for a single crystal with x=0.035 and to 757Â MHz for a film on c-plane sapphire with x=0.001.
ناشر
Database: Elsevier - ScienceDirect (ساینس دایرکت)
Journal: Superlattices and Microstructures - Volume 38, Issues 4â6, OctoberâDecember 2005, Pages 413-420
Journal: Superlattices and Microstructures - Volume 38, Issues 4â6, OctoberâDecember 2005, Pages 413-420
نویسندگان
Mariana Diaconu, Heidemarie Schmidt, Andreas Pöppl, Rolf Böttcher, Joachim Hoentsch, Andreas Rahm, Holger Hochmuth, Michael Lorenz, Marius Grundmann,