Quantitative provenance of silt and clay within sandy deposits of the Lithuanian coastal zone (Baltic Sea)

A quantitative provenance approach is developed and in this study applied for the silt and clay fractions of sandy, coastal deposits. Mineralogical composition of 37 surface samples was determined by X-ray diffraction (XRD). Grain-size distributions were obtained by standard dry sieving and pipette techniques. The characterization of mineralogical provenance is based upon known compositional information of possible sources, logical models for mineral combinations related to regional geological provinces and processes, and geographical features of the documented mineral distribution in the area of investigation. These interpretations are further supported by results of correlation and principal component analyses of mineral varieties, grain-size parameters and bathymetric features of the area. Partitioning of source contributions specific for each site of deposition is derived by solving simultaneous equations. Then, the quantified mineral composition at the initial source is reconstructed in the SE Baltic Sea along the Lithuanian coast, exemplifying this new methodology for quantification of sediment sources. The main sources supplying sediment to the area are: 1) Sambian Peninsula to the south (erosion of Pleistocene till and “Blue Earth” Paleogene sediments), supplying 33% of fine-grained sediment on average, 2) Nemunas River, the discharge of which passes through Curonian Lagoon and supplies an average 17% of the coastal fine sediments, and 3) Pleistocene till, eroded on the sea floor in the north and at the Olando Kepurė shore cliff and contributing an average of 50% of the sediment. Although we use the mineralogy within the environmentally important fine-grained fraction, this mathematically simple approach could be used with any other parameters characterizing the identified sources. A quantification of the separate source contributions to each individual site of accumulation studied, using the stable, mineralogical components of the “sediment archive”, offers a time-integrated, net-effect reflection of the combined processes of an entire environmental system.